Crosby and Nash perform Guinevere, in 1970, one of the finest and most original songs ever conceived IMO. And I generally hate two acoustic + two-part harmony, it's been done to death for decades, but I could listen to this brilliance over and over. The tuning, the meter, the time, the harmony, all are in place and are wonderful.
Apparently Crosby got really high and came up with the guitar tuning for this song. He then proceeded to get amazingly high ever since then but hasn't come up with something this magical.
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